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Mineral grinding often represents a major fraction of total energy costs and coarse pre-concentration can significantly decrease unnecessary processing of barren material. Compressed-air ejection is effective at industrial scale, but suffers from low accuracy at millimeter scale. An opto-magnetic sorting process for coarse pre-concentration of REE-bearing particles before grinding was developed and assessed at labscale. The process combines image-based optical thresholding, water-based wetting of selected particles, magnetite adhesion to wetted surfaces, and magnetic lifting. This process thus couples selective magnetite coating (enabled by localized wetting) and magnetic lifting for particle sorting. The process was run in a reject-oriented mode to facilitate early mass rejection before subsequent comminution. Lab-scale experiments on rauhaugite revealed increasing pre-concentration with decreasing particle size, resulting in a low-grade fraction of 30.4 wt% of the 2–4 mm feed for possible early rejection. The high-grade fraction (57% of the 2–4 mm feed) achieved a TREO concentration of 2.32%, reflecting an enrichment factor of approximately 1.35 compared to the feed (1.71%), consistent with a partial realization of the intrinsic upgrading potential of the ore at this mass yield, as inferred from the TREO distribution of RGB-classified particles. The lab system processed 84 kg/h, corresponding to approximately 1 tonne of feed processed within 12 h. Based on an instantaneous power demand of ∼ 0.8 kW, this corresponds to an energy consumption of ∼ 9.6 kWh/tonne under steady-state conditions. The process also exhibited low water usage (∼5.7 L/tonne feed) and > 99% magnetite recyclability (after 3 runs). Beyond REE beneficiation, the proposed approach shows potential for selective pre-concentration of heterogeneous particulate streams requiring localized actuation. ...
This study presents a method for recovering cement-rich powder from recycled fine aggregates by thermal shock, during which particles are fragmented and spalled due to differential thermal stress. When recycled fine aggregates (RFA) are exposed to high temperatures, the cement paste-rich boundary between the aggregates is weakened and spalled, liberating cement rich particles due to thermal shock. To investigate this phenomenon, experiments have been carried out by subjecting fine recycled aggregates to high temperatures ranging from 500 °C to 700 °C at different residence times. The result suggests that the particles split and crackle due to thermo-mechanical changes. Following thermal treatment, gentle milling completes the liberation process of recycled cement-rich powder (RCP). The composition of the recovered powder confirms the feasibility of the recovery method. To understand the thermo-mechanical process better, modelling efforts have been carried out on a spherical concrete particle of known diameter. The model predicts the temperature profile, residence time and radial stress inside the particle. According to the model, a 2 mm particle experiences a radial stress high enough to overcome the tensile strength of the concrete within 35 s, causing cracks due to the thermal gradient created between the inner and outer surfaces of the particle. These predictions have been verified by experimental results in the laboratory. This approach not only enhances recovery of RCP but also promotes sustainable construction practices. ...
To alleviate the excessive extraction from natural resources and to properly manage construction waste, recycled concrete technology is globally recognized as an eco-friendly way to address these escalating challenges. This study explores the influence of three particle size distributions (PSD) (upper, median, and lower limits) and two curing conditions (normal: 19–25 °C, humidity 48–56 %; lab standard: 20 ± 2 °C, humidity ≥ 95 %) on the compressive strength, tensile splitting strength, and strength development of recycled concrete through a series of experiments. The detailed data make up the research gap in this aspect and reveal that the influence of the PSD on the compressive strength and tensile splitting strength is limited. However, a favourable curing condition benefits the mechanical properties of recycled concrete, especially in resisting tension. In terms of compressive strength, this study indicates that recycled concrete has the potential to replace natural aggregates totally and is feasible to be applied in almost all practical engineering applications, which provides a solid foundation for the future of sustainable construction. ...
Recycled coarse aggregates (RCA) from End-of-Life (EoL) concrete face resistance due to inconsistent quality. To address this, a mobile, containerized sensor-based inspection system is developed, capable of processing over 100 tons of RCA per hour. Using advanced 3D scanning and laser-induced breakdown spectroscopy (LIBS), the system ensures reliable real-time analysis of particle size distribution (PSD) (Root Mean Square Error: <5.5%) and contaminant detection (Accuracy: 0.94). Incremental learning techniques dynamically update chi-square distribution parameters as new spectral data becomes available, refining models continuously without full retraining and sustaining high classification performance. Monitoring data are recorded on radio frequency identification (RFID) tags, enhancing traceability. This innovation improves efficiency compared to traditional methods, supporting sustainable practices in the construction industry. Its applications also extend to related fields such as mining, waste management, and resource recovery, contributing to the circular economy, reducing reliance on natural aggregates, and promoting environmentally friendly infrastructure development. ...
The efficient measurement and optimization of the particle size distribution (PSD) of recycled coarse aggregates (RCA) is critical to ensuring consistent quality in high-performance concrete production. Unlike primary aggregates, which typically demonstrate minimal variability over extended periods and require only occasional testing, RCA often exhibit substantial fluctuations in quality over short timeframes. This variability necessitates a precise, automated, and real-time quality assessment approach, which is lacking in conventional aggregate processing. In this study, a rapid, automated, and non-contact 3D surface analysis method is proposed to assess and optimize the PSD of unscreened RCA during continuous transport on a conveyor belt. A custom-designed conical feeder and splitter facilitate the formation of continuous, symmetric triangular RCA piles, ranging from 4.0 to 16.0 mm in size. Representative PSD measurements are obtained by analyzing a designated strip located at one-third of the pile's height. High-resolution 3D point cloud data are processed using a watershed segmentation algorithm that leverages gradient-based path tracing for efficient topographical mapping. This enables parallel data processing, thereby reducing computational time. The proposed method enables real-time and accurate PSD analysis at industrial throughput levels (≥50 tons per hour) without interrupting conveyor operation, achieving a Root Mean Square Error (RMSE) between 4.69 % and 6.09 %. Furthermore, an optimization strategy based on cumulative percentage retained curves enhances RCA quality and supports continuous process control. The integration of these techniques contributes to improved RCA management and promotes sustainable resource utilization and waste reduction in the construction sector. ...
Journal article (2024) - Lin Wang, Peter Rem, Francesco Di Maio, Max van Beek, Gonçalo Tomás
Solid waste sorting is an important pre-treatment in recycling to improve the efficiency of material recovery and reduce costs. Motivated by the PEACOC project on metal recovery from solid wastes, an innovative magnetic density separation (MDS) process has been developed for solid waste sorting. It has intrinsic advantages over conventional gravity separation technologies and the previously industrialized MDS process. The new MDS process applies an inclined planar magnet and a horizontal basin containing a static magnetic fluid as the separation medium. A particle sliding phenomenon is identified as a feature that could help the separation. Experiments have been carried out to demonstrate the role of the MDS in concentrating valuable metals in shredded PCBAs and reducing metallic contaminants in plastic fractions of shredded wires. A pilot scale facility is introduced to show the design to achieve continuous production and to reduce the consumption of ferrofluid. ...
Conference paper (2024) - Max C. van Beek, Yongli Wu, Peter Rem
Critical raw materials (CRMs) are one of the enablers of a sustainable future due to their importance in green technologies. Yet, their own circularity and end-of-life recycling rates have been lacking as their concentrations are too low in waste products to be efficiently recycled. This is not the case, however, for discarded printed circuit boards where different types of electronics components (ECs) use specific CRMs in high concentrations. Furthermore, due to worldwide manufacturing standards these ECs are consistent between different printed circuit boards (PCBs) in their physical characteristics such as size, shape and material composition. Yet at the moment no sorting methods exist that can separate ECs from modern PCBs. Therefore, we aim to evaluate multiple simple yet effective mechanical separation methods to sort said ECs with CRM recovery in mind. First of all, ECs from flat-panel displays were sieved into a small (<4 mm), medium (4 - 10 mm) and large fraction (>10 mm). This was followed by a roll sorter to separate thinner components, like IC chips, from similarly sized thicker ECs. In order to separate the components based on ferromagnetic composition an innovative overbelt ferromagnetic separator was developed where the magnetic field strength continuously decreased over the length of the belt. Lastly, the different types of ECs were analysed by laser-induced breakdown spectroscopy to identify the presence of any CRMs. Our study shows that by combining these three different sorting technologies it is possible to sort the ECs in a way that the majority of CRM containing components are concentrated in only 21.09 wt% of the total weight. This in turn results in significantly higher CRM concentrations, thus removing a major limitation to their recovery and improving CRM circularity for a more sustainable future.
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Journal article (2024) - Yongli Wu, Tijmen Oudshoorn, Rik Mulder, Kees Van Beek, Peter Rem
The high-precision scrap sorting for effective metal recycling can bring substantial environmental and economic benefits. This article presents a magnetic image sensor that can help to identify the ferrous contaminants inside nonferrous scraps of large sizes. First, the concept and the theory for detecting ferrous contaminants are described. In particular, an inversion algorithm is proposed to characterize the size and position of ferrous contaminants inside the main scrap bodies. Then, based on computed and measured results, the feasibility of sensor design using either 1-D Hall arrays or 1-D pickup coils is demonstrated. Finally, methods are suggested to minimize disturbing signals from very large nonferrous pieces passing through the slightly uneven magnetic field. The obtained findings in this study may apply not only to nonferrous scraps but many other materials of which the mass ratio of the ferrous contaminant to the main material is small. ...
The construction industry urgently requires a resilient information system for effective coordination of data transmission among various stakeholders, including both the public and private sectors. Such an advanced digital solution would not only enhance transparency along the value chain but also improve both the quality of and confidence in recycled materials. Achieving circularity and reducing environmental impact are closely tied to the efficient management of material flows and life cycles. Within this context, Material Passports (MPs) are posited as a foundational element, particularly when integrated with a digital database. This integration is particularly beneficial for increasing the circularity of concrete, beginning with end-of-life concrete, a major contributor to global construction and demolition waste. MPs effectively transmit crucial information about the quality of recycled aggregates, thereby enabling their use in future construction projects. This study explores the feasibility of employing Radio Frequency Identification (RFID) technology as an MP, aiming to enhance sustainability in the concrete industry by improving transparency, traceability, and data reliability in the recycled concrete supply chain. Extensive laboratory tests carried out in three distinct experimental phases revealed that RFID tags exhibit remarkable resilience to mechanical stress typical in the supply chain and consistently maintain readability when embedded in concrete. The water content in concrete samples was identified as a significant factor influencing initial tag readability, although readability improved over time. Other factors, such as the type of aggregates, particle size distribution, and proximity to steel rebar, had minimal to modest impacts on tag performance. Additionally, the study confirmed that the readability of RFID tags remains robust at typical transport speeds, which highlights the potential of an RFID-based system in advancing supply chain management. This study provides a solid foundation for future research in this evolving area. ...

Multi-sensor integration for advanced contaminant detection

Recycling coarse aggregates from construction and demolition waste is essential for sustainable construction practices. However, the quality of recycled coarse aggregates (RCA) often fluctuates significantly, in contrast to the more stable quality of natural aggregates. Contaminants in RCA notably compromise its quality and usability. Therefore, automating the quality control of RCA is necessary for the recycling industry. This study introduces an industry-focused, innovative, and rapid quality control system that combines Laser-Induced Breakdown Spectroscopy (LIBS) with 3D scanning technologies to enhance the detection of contaminants in RCA streams. The system involves a synchronized application of LIBS for spectral analysis and 3D scanning for the physical characterization of different materials. Results reveal that the dependability of single-shot LIBS analysis has been enhanced, thus elevating the precision of contaminant detection. This improvement is achieved by accounting for the laser shot's angle of incidence and focal length adjustments. The introduced technology holds potential for application in the real-time examination of substantial volumes of RCA, facilitating a rapid and reliable quality control method. This rapid assessment technique delivers online data about the concentration of contaminants in RCA, including recycled fine aggregates, cement paste, bricks, foam, glass, gypsum, mineral fibers, plastics, and wood. This data is both essential and sufficient for choosing a cost-effective mortar recipe and guaranteeing the performance of the final concrete product in terms of strength and durability in construction projects. The system can monitor the quality of RCA flows at throughputs of 50 tons per hour per conveyor, characterizing approximately 4000 particles in every ton of RCA, in this way signaling the most critical contaminants at levels of less than 50 parts per million. With these characteristics, the system could also become relevant for other applications, such as characterizing mining waste or solid biofuels for power plants. ...
Journal article (2024) - Ali Vahidi, Arsalan Mostaani, Abraham Teklay Gebremariam, Francesco Di Maio, Peter Rem
This study addresses a critical gap in circular construction practices by assessing the use of high-quality Recycled Coarse Aggregates (RCA) from end-of-life concrete on an industrial scale. Unlike previous studies, which predominantly relied on theoretical mix designs or laboratory-level experiments, this research focuses on real-world applicability, employing commercially produced RCA and conventional production methods in industrial settings to identify upscaling challenges. Advanced Dry Recovery technology is utilized to produce high-quality RCA for both ready-mix and prefab concrete production. To ensure practical relevance, the research examines three water-to-cement ratios for ready-mix concrete and three strength classes for prefab concrete, all prepared and cast in a commercial setting using standard industrial practices. The results show that by selecting the appropriate application for RCA, there is potential for concrete companies to produce mixes using 100% RCA that meet standard requirements in terms of fresh, mechanical, and durability properties without the need for extra treatments or specific mixing methods, particularly when the water absorption of RCA is less than 4%. Achieving optimal performance requires adjustments in the mix design, specifically by considering the effective water-to-cement ratio. Additionally, the study underscores the impact of the parent concrete's properties on the RCA quality. This research not only demonstrates the feasibility of employing RCA in industrial-scale concrete production along with its associated challenges but also highlights the potential for enhancing circularity in the construction industry through large-scale adoption of RCA, thereby contributing to sustainable and circular construction practices. ...
Journal article (2024) - Yongli Wu, Tijmen Oudshoorn, Peter Rem
The growing demand for aluminium worldwide makes aluminium recycling critical to realising a circular economy and increasing the sustainability of our world. One effective way to improve the impact of aluminium recycling is to develop cost-efficient automated sorting technologies for obtaining pre-defined high-quality aluminium scrap products, thus reducing undesirable downcycling and increasing environmental/economic benefits. In this work, an innovative facility, which includes singulation, sensor scanning, and ejection, is optimised for the automated sorting of aluminium scraps. The sorting facility is computationally studied by a virtual experiment model based on the discrete element method. The model considers particle-scale dynamics of complex-shaped scraps and mimics the automated operation of the facility. Based on virtual experiment modelling, the flow of scrap is optimized by computation, with the feasible operation of the sorting facility being proposed. Accordingly, the sorting facility has been built and model predictions are confirmed in actual operation. ...
Journal article (2022) - Cheng Chang, Francesco Di Maio, Peter Rem, Abraham T. Gebremariam, Fanuel Mehari, Han Xia
To upcycle End-of-Life (EoL) concrete from demolished buildings, it is essential to efficiently identify the different materials that may contaminate it. The precise identification and classification of materials and contaminants are vital processes for in-line quality inspection of recycled concrete aggregates transported on a conveyor belt. In this study, a total of eight potential contaminants are considered as target contaminant materials in the streams made of coarse and fine aggregates resulting from the upcycling of EoL concrete. These contaminants degrade the quality of the aggregates even at low concentrations, so it is essential to identify the presence of such contaminants along with the main products of recycling which are recycled coarse aggregates (RCA) and recycled fine aggregates (RFA). An efficient method is proposed to identify and classify EoL concrete waste along with RCA and RFA in motion on conveyor belts via laser-induced breakdown spectroscopy (LIBS) coupled with a cluster-based identification algorithm. The model is verified with an accuracy of 0.97, a precision (weighted average) of 0.98, a recall (weighted average) of 0.97, and an F1-score (weighted average) of 0.98 for the validation set, under the optimal conditions. This study suggests that LIBS may be well suited for fast and in-line analysis of recycled concrete aggregates in industrial applications. This approach presents an innovative approach for the quality characterization of secondary materials produced from EoL concrete being transported on conveyor belts, and therefore can be of great value for the processing and high-end utilization of EoL concrete. ...

Review of Main Current Approaches and Strategic Propositions for an Efficient Circular Economy of Materials

This paper aims to summarize, propose, and discuss existing or emerging strategies to shift towards a circular economy of materials. To clarify the landscape of existing circular practices, a new spectrum is proposed, from product-based strategies, where entire products go through several life cycles without being reprocessed, to material-based approaches, extracting, recycling, and reprocessing materials from the waste flow. As refillable packaging does not lose any functionality or value, when re-used through many life cycles, product-based strategies are globally extremely efficient and must be promoted. It appears however that their implementation is only possible at the scale of individual products such as packaging containers, relying on the cooperation of involved companies and consumers. It appears more and more urgent to focus as well on a more systematic and flexible material-oriented scheme. The example of circular glass recycling is a success in many countries, and technologies become nowadays available to extend such practices to many other materials, such as rigid plastics. An ideal would be to aim at an economy of materials that would imitate the continuous material cycle of the biosphere. Technological and business strategies are presented and discussed, aiming at a relevant impact on circularity. ...
Journal article (2021) - Pingping Wen, Guus Lohlefink, Peter Rem
Can random deposition create dense non-overlapping material feeding? The question is very fundamental for the research of particle packing, while the answer is of great importance for any industrial process that applies single object operation. To gain an insight into this issue, we studied the overlap problems of convex particles in the manner of uniformly random deposition. The overlap probability of two convex particles with arbitrary shapes and sizes is formulated, and the coverage fractions of free particles and sticking particles (particles of the bottom layer) are precisely predicted. Simulations with rectangular particles verified the theory. Surprisingly, free particles can only occupy less than 7.5% of the plane area, much smaller than what is intuitively expected. Sticking particles, however, can easily cover 19%, a factor of 2.5 times larger. The finding is of great value for applications that need to create dense non-overlapping feeding. ...
Journal article (2021) - Abraham T. Gebremariam, Ali Vahidi, Francesco Di Maio, J. Moreno-Juez, I. Vegas-Ramiro, Artur Łagosz, Radosław Mróz, Peter Rem
This study focuses on formulating the most sustainable concrete by incorporating recycled concrete aggregates and other products retrieved from construction and demolition (C&D) activities. Both recycled coarse aggregates (RCA) and recycled fine aggregates (RFA) are firstly used to fully replace the natural coarse and fine aggregates in the concrete mix design. Later, the cement rich ultrafine particles, recycled glass powder and mineral fibres recovered from construction and demolition wastes (CDW) are further incorporated at a smaller rate either as cement substituent or as supplementary additives. Remarkable properties are noticed when the RCA (4–12 mm) and RFA (0.25–4 mm) are fully used to replace the natural aggregates in a new concrete mix. The addition of recycled cement rich ultrafines (RCU), Recycled glass ultrafines (RGU) and recycled mineral fibres (RMF) into recycled concrete improves the modulus of elasticity. The final concrete, which comprises more than 75% (wt.) of recycled components/materials, is believed to be the most sustainable and green concrete mix. Mechanical properties and durability of this concrete have been studied and found to be within acceptable limits, indicating the potential of recycled aggregates and other CDW components in shaping sustainable and circular construction practices. ...
Journal article (2021) - J.J. Kosse, M. Dhallé, P.C. Rem, H.J.M. ter Brake, H.H.J. ten Kate
In this article, electromagnet layouts are presented, which generate a magnetic field with a magnitude gradient that does not vary significantly in a horizontal plane but decreases monotonically with the vertical height above the magnet. Such a one-direction magnetic field gradient is a specific requirement for magnetic density separation (MDS), a novel recycling technology that combines a vertical magnetic field gradient with a ferrofluid to separate a mixture of non-magnetic materials based on their mass density. We are assembling the first superconducting magnet to be used for this application. In contrast to other separation technologies that use ferrofluid, multiple products can be separated in a single process step. First, the idealized current distribution is introduced that produces such a magnetic field with a magnitude that decays only in one direction. This ideal field can be approximated with practical coil configurations, which are evaluated with a Fourier analysis to derive an optimal cross-sectional layout based on flat racetrack coils. The analysis concludes with a discussion of the effect of winding pack thickness on the value of the magnetic field above the magnet system and the peak field inside the winding pack. The conclusions of this study are applicable not just for MDS but for any application that requires a magnetic field gradient that changes only in one direction. ...
Journal article (2021) - J.J. Kosse, M. Dhallé, G. Tomás, P.C. Rem, H.J.M. ter Brake, H.H.J. ten Kate
This article discusses the optimum layout of coils of a superconducting magnet system for magnetic density separation (MDS). MDS is a novel separation technology that combines a vertical magnetic field gradient with a ferrofluid to separate mixtures of non-magnetic particles based on their mass density. The MDS process can separate more than two types of particles in a single process step, thereby distinguishing it from other separation techniques using a ferrofluid. The authors are currently constructing a superconducting MDS demonstrator. Ideally, the gradient of the magnetic field magnitude should change only with the distance above the magnet but remain constant in a horizontal plane. In principle, such an ideal field profile can be generated with an infinite harmonic sheet current. In practice, edge effects appear due to the necessity of using a finite number of coils. These cause a horizontal component in the field gradient and also change the vertical component. We compare the vertical magnetic field gradient of various coil layouts to see which configuration performs best. To facilitate ease of production, the analysis is restricted to flat racetrack coils. The main result is that the specific shape of a racetrack coil has a larger influence on the vertical gradient than the number of coils. The feed particles need to be pushed through the separation chamber from the insertion to the collection point. One option to realize this is to use an MDS setup in which the magnet is inclined with respect to the horizontal plane. This tilting results in a horizontal magnetic force component, which drives feed particles through the fluid bed. We show that a three-coil layout provides the largest usable fluid bed depth for a wide range of tilt angles. ...
Currently, natural resources are consumed at an alarming rate than their production (United Nations Environment Programme, 2014). This imposes unprecedented pressure on the environment. The problem seems to get worse with the present increase in population and demand for infrastructures. To alleviate these and other related problems, a circular approach to construction material flow is crucial. Recycling construction and demolition wastes (C&DW) to generate high-quality materials is essential to ensure materials circularity in the construction sector. This article, therefore, describes the development of two large-scale technologies called Advanced Dry Recovery (ADR) and Heating Air classification System (HAS). ADR and HAS are industrial-scale technologies aimed to recycle End-of-Life (EoL) concrete into coarse, fine and ultrafine particles. While ADR is used to sort out clean coarse aggregates, HAS is used to produce clean fine aggregates by heating and separating the ultrafine hydrated cement components. The process parameters and the quality of aggregates are briefly described. Accordingly, concrete made of recycled coarse and fine aggregates displays comparable mechanical properties as the reference concrete which is made of natural aggregates. Both technologies are designed to be mobile so that EoL concrete wastes are processed at the site of demolition or close to ready-mix concrete plants, reducing the heavy traffic related to construction activities. These technologies, in general, have a potential in increasing sustainability and thereby greening the construction sector. This is by far a convenient contribution towards sustainable development and a big step towards closing the recycling loop in the construction sector. ...