D. Bouman
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Retraction Note - Epitaxy of advanced nanowire quantum devices
Correction to: Nature https://doi.org/10.1038/nature23468 Published online 24 August 2017
The authors of the paper “Epitaxy of advanced nanowire quantum devices”1 wish to retract this work. When preparing the underlying data for public release2, it was discovered that some data had been inappropriately deleted or cropped when preparing the final published figures, and we promptly alerted the editors of Nature. We found unjustified data removal and cropping in Figures 4a and c, and Extended Data Figures 7 and 8, which affect the agreement between the theoretical curves and the experimental data and the claims of ballistic transport. We are accordingly retracting the paper. The authors stand by all the other data, and their contribution to advanced nanowire quantum devices. All authors have agreed to this retraction.
Electrostatic charging affects the many-body spectrum of Andreev states, yet its influence on their microwave properties has not been elucidated. We developed a circuit quantum electrodynamics probe that, in addition to transition spectroscopy, measures the microwave susceptibility of different states of a semiconductor nanowire weak link with a single dominant (spin-degenerate) Andreev level. We found that the microwave susceptibility does not exhibit a particle-hole symmetry, which we qualitatively explain as an influence of Coulomb interaction. Moreover, our state-selective measurement reveals a large, ?-phase shifted contribution to the response common to all many-body states which can be interpreted as arising from a phase-dependent continuum in the superconducting density of states.
Two promising architectures for solid-state quantum information processing are based on electron spins electrostatically confined in semiconductor quantum dots and the collective electrodynamic modes of superconducting circuits. Superconducting electrodynamic qubits involve macroscopic numbers of electrons and offer the advantage of larger coupling, whereas semiconductor spin qubits involve individual electrons trapped in microscopic volumes but are more difficult to link. We combined beneficial aspects of both platforms in the Andreev spin qubit: the spin degree of freedom of an electronic quasiparticle trapped in the supercurrent-carrying Andreev levels of a Josephson semiconductor nanowire. We performed coherent spin manipulation by combining single-shot circuit–quantum-electrodynamics readout and spin-flipping Raman transitions and found a spin-flip time TS = 17 microseconds and a spin coherence time T2E = 52 nanoseconds. These results herald a regime of supercurrent-mediated coherent spin-photon coupling at the single-quantum level.
We measure the charge periodicity of Coulomb blockade conductance oscillations of a hybrid InSb-Al island as a function of gate voltage and parallel magnetic field. The periodicity changes from to at a gate-dependent value of the magnetic field, , decreasing from a high to a low limit upon increasing the gate voltage. In the gate voltage region between the two limits, which our numerical simulations indicate to be the most promising for locating Majorana zero modes, we observe correlated oscillations of peak spacings and heights. For positive gate voltages, the transition with low is due to the presence of nontopological states whose energy quickly disperses below the charging energy due to the orbital effect of the magnetic field. Our measurements highlight the importance of a careful exploration of the entire available phase space of a proximitized nanowire as a prerequisite to define future topological qubits.
Author Correction
Continuous monitoring of a trapped superconducting spin (Nature Physics, (2020), 16, 11, (1103-1107), 10.1038/s41567-020-0952-3)
In this Letter the following original sentence has been amended for clarity: “As the Kramers theorem does not hold in the presence of a non-zero weak-link phase bias φ, the splitting of the spin states requires an additional ingredient.”; it has been changed to: “Although the presence of a non-zero weak-link phase bias φ breaks time-reversal symmetry so that the Kramers theorem does not hold, this alone is insufficient to lift the spin degeneracy—an additional effect is required.” The online versions of the Letter have been amended.
Today, quantum computers are in their infancy and realizing a computer powerful enough to perform useful calculations poses major challenges. The fragility of qubits being the main difficulty. Approaches to mitigate this include implementing error correction schemes or alternative qubit designs. Topological qubits are part of the latter category and exploit the robustness of topologically invariant states to small perturbations to create more stable qubits.
In this thesis we explore semiconductor-superconductor hybrid nanowire structures and in particular the interaction of electron spins in quantum dots with superconductivity. When connected to superconductors, arrays of superconductor quantum dot hybrids can host Majorana states, a promising approach to realizing topological qubits. Creating Majoranas in quantum dots, as opposed to traditional methods, offers greater control over their properties. Additionally, understanding the interaction between spins in these quantum dots superconductor hybrids could enable new readout methods or coupling mechanisms between superconducting and spin qubits.
We start by investigating a nanowire SNS Josephson junction with signatures of Majorana states. A nanowire junction is capacitively coupled to an on-chip microwave detector made from a Josephson tunnel junction. We monitor the Josephson radiation frequency as a function of magnetic field and find a transition from a $2\pi$ to a $4\pi$-periodic Josephson current-phase relation, consistent with a topological transition.
In a different device, we investigate a multi-orbital double quantum dot Josephson junction. We measure the excitations between doublet and singlet states that arise in a quantum dot weakly coupled to a superconducting lead, also known as Yu-Shiba-Rusinov (YSR) states. With increased dot-lead coupling we observe a supercurrent and reveal its current-phase relation, both in the single and multi-orbit regime. We show that in the single-orbital regime the supercurrent sign follows an even-odd charge occupation effects. In the even charge parity sector, we observe a supercurrent blockade when the spin ground state transitions to a triplet -- demonstrating a direct spin to supercurrent conversion. For yet stronger dot-lead coupling we find a rectified current-phase relation at the transition between even and odd charge states. We investigate this apparent non-equilibrium effect and think about possible explanations.
To conclude, we discuss possible applications in spin qubit state readout and extensions of the device geometry towards realizing a Kiteav chain able to host Majorana states. ...
Today, quantum computers are in their infancy and realizing a computer powerful enough to perform useful calculations poses major challenges. The fragility of qubits being the main difficulty. Approaches to mitigate this include implementing error correction schemes or alternative qubit designs. Topological qubits are part of the latter category and exploit the robustness of topologically invariant states to small perturbations to create more stable qubits.
In this thesis we explore semiconductor-superconductor hybrid nanowire structures and in particular the interaction of electron spins in quantum dots with superconductivity. When connected to superconductors, arrays of superconductor quantum dot hybrids can host Majorana states, a promising approach to realizing topological qubits. Creating Majoranas in quantum dots, as opposed to traditional methods, offers greater control over their properties. Additionally, understanding the interaction between spins in these quantum dots superconductor hybrids could enable new readout methods or coupling mechanisms between superconducting and spin qubits.
We start by investigating a nanowire SNS Josephson junction with signatures of Majorana states. A nanowire junction is capacitively coupled to an on-chip microwave detector made from a Josephson tunnel junction. We monitor the Josephson radiation frequency as a function of magnetic field and find a transition from a $2\pi$ to a $4\pi$-periodic Josephson current-phase relation, consistent with a topological transition.
In a different device, we investigate a multi-orbital double quantum dot Josephson junction. We measure the excitations between doublet and singlet states that arise in a quantum dot weakly coupled to a superconducting lead, also known as Yu-Shiba-Rusinov (YSR) states. With increased dot-lead coupling we observe a supercurrent and reveal its current-phase relation, both in the single and multi-orbit regime. We show that in the single-orbital regime the supercurrent sign follows an even-odd charge occupation effects. In the even charge parity sector, we observe a supercurrent blockade when the spin ground state transitions to a triplet -- demonstrating a direct spin to supercurrent conversion. For yet stronger dot-lead coupling we find a rectified current-phase relation at the transition between even and odd charge states. We investigate this apparent non-equilibrium effect and think about possible explanations.
To conclude, we discuss possible applications in spin qubit state readout and extensions of the device geometry towards realizing a Kiteav chain able to host Majorana states.
Serial double quantum dots created in semiconductor nanostructures provide a versatile platform for investigating two-electron spin quantum states, which can be tuned by electrostatic gating and an external magnetic field. In this Rapid Communication, we directly measure the supercurrent reversal between adjacent charge states of an InAs nanowire double quantum dot with superconducting leads, in good agreement with theoretical models. In the even charge parity sector, we observe a supercurrent blockade with increasing magnetic field, corresponding to the spin singlet to triplet transition. Our results demonstrate a direct spin to supercurrent conversion, the superconducting equivalent of the Pauli spin blockade. This effect can be exploited in hybrid quantum architectures coupling the quantum states of spin systems and superconducting circuits.
Readout and control of electrostatically confined electrons in semiconductors are key primitives of quantum information processing with solid-state spin qubits1,2. In superconductor–semiconductor heterostructures, localized electronic modes known as Andreev levels result from confinement that is provided by the pair potential3,4. Unlike electronic modes confined exclusively via electrostatic effects, Andreev levels carry supercurrent. Therefore, they naturally integrate with the techniques of circuit quantum electrodynamics (cQED) that have been developed in the field of superconducting qubits and used to detect pairs of quasiparticles that are trapped in Andreev levels5–8. Here, we demonstrate single-shot cQED readout of the spin of an individual quasiparticle trapped in the Andreev levels of a semiconductor nanowire Josephson element. Owing to a spin-orbit interaction in the nanowire, this ‘superconducting spin’ directly determines the flow of supercurrent through the element. We harnessed this spin-dependent supercurrent to achieve both a zero-field spin splitting and a long-range interaction between the quasiparticle and a superconducting microwave resonator9–13. Measurement of the resultant spin-dependent resonator frequency yielded quantum non-demolition spin readout with 92% fidelity in 1.9 μs, which enabled us to monitor the quasiparticle spin in real time. These results pave the way for superconducting spin qubits that operate at zero magnetic field and for time-domain measurements of Majorana zero modes9,10,12,14,15.
Quantum computation by non-Abelian Majorana zero modes (MZMs) offers an approach to achieve fault tolerance by encoding quantum information in the non-local charge parity states of semiconductor nanowire networks in the topological superconductor regime. Thus far, experimental studies of MZMs chiefly relied on single electron tunneling measurements, which lead to the decoherence of the quantum information stored in the MZM. As a next step towards topological quantum computation, charge parity conserving experiments based on the Josephson effect are required, which can also help exclude suggested non-topological origins of the zero bias conductance anomaly. Here we report the direct measurement of the Josephson radiation frequency in indium arsenide nanowires with epitaxial aluminium shells. We observe the 4π-periodic Josephson effect above a magnetic field of ≈200 mT, consistent with the estimated and measured topological phase transition of similar devices.
The modern understanding of the Josephson effect in mesosopic devices derives from the physics of Andreev bound states, fermionic modes that are localized in a superconducting weak link. Recently, Josephson junctions constructed using semiconducting nanowires have led to the realization of superconducting qubits with gate-tunable Josephson energies. We have used a microwave circuit QED architecture to detect Andreev bound states in such a gate-tunable junction based on an aluminum-proximitized indium arsenide nanowire. We demonstrate coherent manipulation of these bound states, and track the bound-state fermion parity in real time. Individual parity-switching events due to nonequilibrium quasiparticles are observed with a characteristic timescale Tparity=160±10 μs. The Tparity of a topological nanowire junction sets a lower bound on the bandwidth required for control of Majorana bound states.
The number of electrons in small metallic or semiconducting islands is quantised. When tunnelling is enabled via opaque barriers this number can change by an integer. In superconductors the addition is in units of two electron charges (2e), reflecting that the Cooper pair condensate must have an even parity. This ground state (GS) is foundational for all superconducting qubit devices. Here, we study a hybrid superconducting-semiconducting island and find three typical GS evolutions in a parallel magnetic field: a robust 2e-periodic even-parity GS, a transition to a 2e-periodic odd-parity GS, and a transition from a 2e- to a 1e-periodic GS. The 2e-periodic odd-parity GS persistent in gate-voltage occurs when a spin-resolved subgap state crosses zero energy. For our 1e-periodic GSs we explicitly show the origin being a single zero-energy state gapped from the continuum, i.e., compatible with an Andreev bound states stabilized at zero energy or the presence of Majorana zero modes.
Semiconductor nanowires are ideal for realizing various low-dimensional quantum devices. In particular, topological phases of matter hosting non-Abelian quasiparticles (such as anyons) can emerge when a semiconductor nanowire with strong spin-orbit coupling is brought into contact with a superconductor. To exploit the potential of non-Abelian anyons - which are key elements of topological quantum computing - fully, they need to be exchanged in a well-controlled braiding operation. Essential hardware for braiding is a network of crystalline nanowires coupled to superconducting islands. Here we demonstrate a technique for generic bottom-up synthesis of complex quantum devices with a special focus on nanowire networks with a predefined number of superconducting islands. Structural analysis confirms the high crystalline quality of the nanowire junctions, as well as an epitaxial superconductor-semiconductor interface. Quantum transport measurements of nanowire 'hashtags' reveal Aharonov-Bohm and weak-antilocalization effects, indicating a phase-coherent system with strong spin-orbit coupling. In addition, a proximity-induced hard superconducting gap (with vanishing sub-gap conductance) is demonstrated in these hybrid superconductor-semiconductor nanowires, highlighting the successful materials development necessary for a first braiding experiment. Our approach opens up new avenues for the realization of epitaxial three-dimensional quantum architectures which have the potential to become key components of various quantum devices.
The superconducting proximity effect in semiconductor nanowires has recently enabled the study of new superconducting architectures, such as gate-tunable superconducting qubits and multiterminal Josephson junctions. As opposed to their metallic counterparts, the electron density in semiconductor nanosystems is tunable by external electrostatic gates, providing a highly scalable and in situ variation of the device properties. In addition, semiconductors with large g-factor and spin-orbit coupling have been shown to give rise to exotic phenomena in superconductivity, such as † 0 Josephson junctions and the emergence of Majorana bound states. Here, we report microwave spectroscopy measurements that directly reveal the presence of Andreev bound states (ABS) in ballistic semiconductor channels. We show that the measured ABS spectra are the result of transport channels with gate-tunable, high transmission probabilities up to 0.9, which is required for gate-tunable Andreev qubits and beneficial for braiding schemes of Majorana states. For the first time, we detect excitations of a spin-split pair of ABS and observe symmetry-broken ABS, a direct consequence of the spin-orbit coupling in the semiconductor.