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L.J. Feije

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Solid-state spin defects are promising qubits for quantum network nodes. A key challenge toward larger networks is creating defects with high yield into nanophotonic devices while maintaining good optical and spin properties. Here, we demonstrate the creation of single V2 centers in nanopillars fabricated from commercial bulk-grown 4H-silicon carbide using a pulsed above-bandgap (UV) laser. We observe an 11-fold increase in the V2 center occurrence after UV laser illumination. These laser-induced V2 centers exhibit narrow optical line widths and spectral diffusion rates comparable to naturally occurring V2 centers in nanopillars of the same material. Furthermore, we measure a spin coherence time of (Formula presented) under dynamical decoupling, consistent with dephasing by the nuclear-spin bath. This demonstration of the in situ, postfabrication generation of coherent V2 centers in nanostructures in widely available bulk-grown 4H-SiC shows the potential for above-bandgap laser illumination for scalable defect creation in integrated photonic devices. ...
Solid-state single-photon emitters provide a versatile platform for exploring quantum technologies such as optically connected quantum networks. A key challenge is to ensure the optical coherence and spectral stability of the emitters. Here, we introduce a high-bandwidth ‘check-probe’ scheme to quantitatively measure (laser-induced) spectral diffusion and ionisation rates, as well as homogeneous linewidths. We demonstrate these methods on single V2 centres in commercially available bulk-grown 4H-silicon carbide. Despite observing significant spectral diffusion under laser illumination (≳GHz s−1), the optical transitions are narrow (~35 MHz), and remain stable in the dark (≳1 s). Through Landau-Zener-Stückelberg interferometry, we determine the optical coherence to be near-lifetime limited (T2 = 16.4(4) ns), hinting at the potential for using bulk-grown materials for developing quantum technologies. These results advance our understanding of spectral diffusion of quantum emitters in semiconductor materials, and may have applications for studying charge dynamics across other platforms. ...
We demonstrate coherent coupling of a single diamond Tin-Vacancy center to a fiber-based microcavity, showing a cavity transmission dip of 50 % on resonance, and altered photon statistics in cavity transmission. ...
We report on the realization of a fiber-based microcavity, exhibiting low cavity length fluctuations in combination with full spatial and spectral tunability. The microcavity is used to demonstrate Purcell-enhancement of diamond Tin-Vacancy centers. ...
Open microcavities offer great potential for the exploration and utilization of efficient spin-photon interfaces with Purcell-enhanced quantum emitters thanks to their large spectral and spatial tunability combined with high versatility of sample integration. However, a major challenge for this platform is the sensitivity to cavity length fluctuations in the cryogenic environment, which leads to cavity resonance frequency variations and thereby a lowered averaged Purcell enhancement. This work presents a closed-cycle cryogenic fiber-based microcavity setup, which is in particular designed for a low passive vibration level, while still providing large tunability and flexibility in fiber and sample integration, and high photon collection efficiency from the cavity mode. At temperatures below 10 K, a stability level of around 25 pm is reproducibly achieved in different setup configurations, including the extension with microwave control for manipulating the spin of cavity-coupled quantum emitters, enabling a bright photonic interface with optically active qubits. ...
Efficient coupling of optically active qubits to optical cavities is a key challenge for solid-state-based quantum optics experiments and future quantum technologies. Here we present a quantum photonic interface based on a single tin-vacancy center in a micrometer-thin diamond membrane coupled to a tunable open microcavity. We use the full tunability of the microcavity to selectively address individual tin-vacancy centers within the cavity mode volume. Purcell enhancement of the tin-vacancy center optical transition is evidenced both by optical excited state lifetime reduction and by optical linewidth broadening. As the emitter selectively reflects the single-photon component of the incident light, the coupled emitter-cavity system exhibits strong quantum nonlinear behavior. On resonance, we observe a transmission dip of 50% for low incident photon number per Purcell-reduced excited state lifetime, while the dip disappears as the emitter is saturated with higher photon number. Moreover, we demonstrate that the emitter strongly modifies the photon statistics of the transmitted light by observing photon bunching. This work establishes a versatile and tunable platform for advanced quantum optics experiments and proof-of-principle demonstrations on quantum networking with solid-state qubits. ...
We show diamond Tin-Vacancy centers, coherently-coupled to a tunable microcavity. The exceptional optical properties of this emitter in combination with a stable, high quality cavity enables a cavity transmission signal modulated by a single emitter. ...