Solid-state quantum registers consisting of optically active electron spins with nearby nuclear spins are promising building blocks for future quantum technologies. For electron spin-1 registers, dynamical decoupling (DD) quantum gates have been developed that enable the precise control of multiple nuclear spin qubits. However, for the important class of electron spin-1/2 systems, this control method suffers from intrinsic selectivity limitations, resulting in reduced nuclear spin gate fidelities. Here, we demonstrate improved control of single nuclear spins by an electron spin-1/2 using dynamically decoupled radio-frequency (DDRF) gates. We make use of the electron spin-1/2 of a diamond tin-vacancy center, showing high-fidelity single-qubit gates, single-shot readout, and spin coherence beyond a millisecond. The DD control is used as a benchmark to observe and control a single 31C nuclear spin. Using the DDRF control method, we demonstrate improved control on that spin. In addition, we find and control an additional nuclear spin that is insensitive to the DD control method. Using these DDRF gates, we show entanglement between the electron and the nuclear spin with 72(3)% state fidelity. Our extensive simulations indicate that DDRF gate fidelities well in excess are feasible. Finally, we employ time-resolved photon detection during readout to quantify the hyperfine coupling for the electron's optically excited state. Our work provides key insights into the challenges and opportunities for nuclear spin control in electron spin-1/2 systems, opening the door to multiqubit experiments on these promising qubit platforms.

We demonstrate large-range tuning of the optical transition of Tin-Vacancies (SnV) in diamond using electro-mechanical-induced strain, realizing >40 GHz tuning. We employ real-time feedback on the strain environment to stabilize the resonant frequency.

Diamond photonic crystal cavity parameters are measured at cryogenic temperatures. In-situ resonance frequency tuning through gas desorption allows us to probe the SnV-cavity system.

Quantum networks are based on shared remote entanglement between local nodes by exchanging indistinguishable photons. We show Two-Photon Quantum Interference between tin-vacancy centers in diamond-waveguides and report on the progress towards remote entanglement generation.

The negatively charged tin-vacancy (SnV⁻) center in diamond has emerged as a promising platform for quantum computing and quantum networks. To connect SnV⁻ qubits in large networks, in situ tuning and stabilization of their optical transitions are essential to overcome static and dynamic frequency offsets induced by the local environment. Here, we report on the large-range optical frequency tuning of diamond SnV⁻ centers using micro-electro-mechanically mediated strain control in photonic integrated waveguide devices. We realize a tuning range of >40 GHz, covering a major part of the inhomogeneous distribution. In addition, we employ real-time feedback on the strain environment to stabilize the resonance frequency and mitigate spectral wandering. These results provide a path for on-chip scaling of diamond SnV-based quantum networks.

Micrometer-scale thin diamond devices are key components for various quantum sensing and networking experiments, including the integration of color centers into optical microcavities. In this work, we introduce a laser-cutting method for patterning microdevices from millimeter-sized diamond membranes. The method can be used to fabricate devices with micrometer thicknesses and edge lengths of typically 10-100 µm. We compare this method with an established nanofabrication process based on electron-beam lithography, a two-step transfer pattern utilizing a silicon nitride hard mask material, and reactive ion etching. Microdevices fabricated using both methods are bonded to a cavity Bragg mirror and characterized using scanning cavity microscopy. We record two-dimensional cavity finesse maps over the devices, revealing insights about the variation in diamond thickness, surface quality, and strain. The scans demonstrate that devices fabricated by laser-cutting exhibit similar properties to devices obtained by the conventional method. Finally, we show that the devices host optically coherent Tin- and Nitrogen-Vacancy centers suitable for applications in quantum networking.

Color centers integrated with nanophotonic devices have emerged as a compelling platform for quantum science and technology. Here, we integrate tin-vacancy centers in a diamond waveguide and investigate the interaction with light at the single-photon level in both reflection and transmission. We observe single-emitter-induced extinction of the transmitted light up to 25% and measure the nonlinear effect on the photon statistics. Furthermore, we demonstrate fully tunable interference between the reflected single-photon field and laser light backscattered at the fiber end and show the corresponding controlled change between bunched and antibunched photon statistics in the reflected field.

We show coupling of an SnV center to a diamond waveguide of 20% with almost transform-limited optical transitions. Besides, we show control over the SnV spin qubit and extend its coherence to over a millisecond.

Open microcavities offer great potential for the exploration and utilization of efficient spin-photon interfaces with Purcell-enhanced quantum emitters thanks to their large spectral and spatial tunability combined with high versatility of sample integration. However, a major challenge for this platform is the sensitivity to cavity length fluctuations in the cryogenic environment, which leads to cavity resonance frequency variations and thereby a lowered averaged Purcell enhancement. This work presents a closed-cycle cryogenic fiber-based microcavity setup, which is in particular designed for a low passive vibration level, while still providing large tunability and flexibility in fiber and sample integration, and high photon collection efficiency from the cavity mode. At temperatures below 10 K, a stability level of around 25 pm is reproducibly achieved in different setup configurations, including the extension with microwave control for manipulating the spin of cavity-coupled quantum emitters, enabling a bright photonic interface with optically active qubits.

We demonstrate heralded initialization of charge state and optical transition frequency of diamond tin-vacancy centers, using (off-)resonant lasers, photon detection and real-time logic. Using this, we show frequency tunability > 100 MHz and strongly improved optical coherence.

We demonstrate coherent coupling of a single diamond Tin-Vacancy center to a fiber-based microcavity, showing a cavity transmission dip of 50 % on resonance, and altered photon statistics in cavity transmission.

We present our optimized diamond fabrication process based on quasi-isotropic crystal-plane-dependent reactive-ion-etching at low and high temperature plasma regime. We demonstrate successful integration of SnV centers in diamond waveguides showing quantum non-linear effects. We report on our latest results on all-diamond photonic crystal cavities.

Diamond tin-vacancy centers have emerged as a promising platform for quantum information science and technology. A key challenge for their use in more-complex quantum experiments and scalable applications is the ability to prepare the center in the desired charge state with the optical transition at a predefined frequency. Here we report on heralding such successful preparation using a combination of laser excitation, photon detection, and real-time logic. We first show that fluorescence photon counts collected during an optimized resonant probe pulse strongly correlate with the subsequent charge state and optical-transition frequency, enabling real-time heralding of the desired state through threshold photon counting. We then implement and apply this heralding technique to photoluminescence-excitation measurements, coherent optical driving, and an optical Ramsey experiment, finding strongly increased optical coherence with increasing threshold. Finally, we demonstrate that the prepared optical frequency follows the probe laser across the inhomogeneous linewidth, enabling tuning of the transition frequency over multiple homogeneous linewidths.

We show diamond Tin-Vacancy centers, coherently-coupled to a tunable microcavity. The exceptional optical properties of this emitter in combination with a stable, high quality cavity enables a cavity transmission signal modulated by a single emitter.

We fabricate single tin-vacancy centres in diamond, we perform spectroscopy and coherent population trapping to verify optical driving of the spin states. We investigate the integration in diamond waveguides to realise an efficient spin-photon interface.