Q. Wang
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In semiconducting-superconducting hybrid devices, Andreev bound states (ABSs) can mediate the coupling between quantum dots, allowing for the realization of artificial Kitaev chains. In order to engineer Majorana bound states (MBSs) in these systems, one must control the energy of the ABSs. In this Letter, we show how extended ABSs in a flux-tunable Josephson junction can be used to control the coupling between distant quantum dots separated by ≃1 μm. In particular, we demonstrate that the combination of electrostatic control and phase control over the ABSs increases the parameter space in which MBSs are observed. Finally, by employing an additional spectroscopic probe in the hybrid region between the quantum dots, we gain information about the spatial distribution of the Majorana wave function in a two-site Kitaev chain.
Their non-Abelian statistics make them promising building blocks for topological quantum computation.
In semiconductor–superconductor hybrids, however, disorder and trivial bound states often obscure Majorana signatures,
making conclusive evidence elusive. This challenge motivates new device concepts or alternative engineering strategies.
In this thesis, we bridge a traditional and a new bottom-up routes to realize Majorana modes in two-dimensional electron gases (2DEGs), and develop a fabrication workflow for complex device geometries.
We first implement the Lutchyn–Oreg approach in gate-defined wires and develop multiprobe spectroscopy with multiple tunnel probes to assess spatial uniformity.
These measurements reveal subgap states that are often uncorrelated between neighboring probes, though some devices show striking probe-to-probe correlations.
These observations indicate that disorder and inhomogeneity can drive inconsistent behavior across similar devices, limiting prospects for a robust global topological phase.
This motivates an alternative pathway: constructing artificial Kitaev chains using quantum dots.In the second experiment, we establish controllable elastic cotunneling and crossed Andreev reflection, via gate-tunable Andreev bound states that couple the dots.
We demonstrate Cooper pair splitting and at finite magnetic field, we are able to resolve substantial triplet correlations due to the strong spin orbit coupling in the 2DEGs.
In the third experiment, we push the system into the strong-coupling regime and realize a two-site Kitaev chain.
By tuning dot levels, the ABS energy, and the in-plane magnetic-field orientation, we reach “sweet spots” with correlated zero-bias peaks that are robust to local perturbations.
Notably, these peaks can already appear at zero Zeeman energy—consistent with a spinful two-site chain.
Comparing the full excitation spectrum to numerical simulations allows us to estimate the Majorana polarization in representative settings.
We conclude this thesis by outlining next steps: extending the Kitaev chain and implementing parity readout to enable manipulation and measurement of multiple MBSs.
We also assess alternative material platforms for proof-of-principle Kitaev-chain devices.
...
Their non-Abelian statistics make them promising building blocks for topological quantum computation.
In semiconductor–superconductor hybrids, however, disorder and trivial bound states often obscure Majorana signatures,
making conclusive evidence elusive. This challenge motivates new device concepts or alternative engineering strategies.
In this thesis, we bridge a traditional and a new bottom-up routes to realize Majorana modes in two-dimensional electron gases (2DEGs), and develop a fabrication workflow for complex device geometries.
We first implement the Lutchyn–Oreg approach in gate-defined wires and develop multiprobe spectroscopy with multiple tunnel probes to assess spatial uniformity.
These measurements reveal subgap states that are often uncorrelated between neighboring probes, though some devices show striking probe-to-probe correlations.
These observations indicate that disorder and inhomogeneity can drive inconsistent behavior across similar devices, limiting prospects for a robust global topological phase.
This motivates an alternative pathway: constructing artificial Kitaev chains using quantum dots.In the second experiment, we establish controllable elastic cotunneling and crossed Andreev reflection, via gate-tunable Andreev bound states that couple the dots.
We demonstrate Cooper pair splitting and at finite magnetic field, we are able to resolve substantial triplet correlations due to the strong spin orbit coupling in the 2DEGs.
In the third experiment, we push the system into the strong-coupling regime and realize a two-site Kitaev chain.
By tuning dot levels, the ABS energy, and the in-plane magnetic-field orientation, we reach “sweet spots” with correlated zero-bias peaks that are robust to local perturbations.
Notably, these peaks can already appear at zero Zeeman energy—consistent with a spinful two-site chain.
Comparing the full excitation spectrum to numerical simulations allows us to estimate the Majorana polarization in representative settings.
We conclude this thesis by outlining next steps: extending the Kitaev chain and implementing parity readout to enable manipulation and measurement of multiple MBSs.
We also assess alternative material platforms for proof-of-principle Kitaev-chain devices.
The formation of a topological superconducting phase in a quantum-dot-based Kitaev chain requires nearest neighbor crossed Andreev reflection and elastic cotunneling. Here, we report on a hybrid InSb nanowire in a three-site Kitaev chain geometry - the smallest system with well-defined bulk and edge - where two superconductor-semiconductor hybrids separate three quantum dots. We demonstrate pairwise crossed Andreev reflection and elastic cotunneling between both pairs of neighboring dots and show sequential tunneling processes involving all three quantum dots. These results are the next step toward the realization of topological superconductivity in long Kitaev chain devices with many coupled quantum dots.
Majorana bound states are expected to appear in one-dimensional semiconductor-superconductor hybrid systems, provided they are homogeneous enough to host a global topological phase. In order to experimentally investigate the uniformity of the system, we study the spatial dependence of the local density of states in multiprobe devices where several local tunneling probes are positioned along a gate-defined wire in a two-dimensional electron gas. Spectroscopy at each probe reveals a hard induced gap and an absence of subgap states at zero magnetic field. However, subgap states emerging at a finite magnetic field are not always correlated between different probes. Moreover, we find that the extracted critical field and effective g-factor vary significantly across the length of the wire. Upon studying several such devices, we do however find examples of striking correlations in the local density of states measured at different tunnel probes. We discuss possible sources of variation across devices.
Cooper pairs occupy the ground state of superconductors and are typically composed of maximally entangled electrons with opposite spin. In order to study the spin and entanglement properties of these electrons, one must separate them spatially via a process known as Cooper pair splitting (CPS). Here we provide the first demonstration of CPS in a semiconductor two-dimensional electron gas (2DEG). By coupling two quantum dots to a superconductor-semiconductor hybrid region we achieve efficient Cooper pair splitting, and clearly distinguish it from other local and non-local processes. When the spin degeneracy of the dots is lifted, they can be operated as spin-filters to obtain information about the spin of the electrons forming the Cooper pair. Not only do we observe a near perfect splitting of Cooper pairs into opposite-spin electrons (i.e. conventional singlet pairing), but also into equal-spin electrons, thus achieving triplet correlations between the quantum dots. Importantly, the exceptionally large spin-orbit interaction in our 2DEGs results in a strong triplet component, comparable in amplitude to the singlet pairing. The demonstration of CPS in a scalable and flexible platform provides a credible route to study on-chip entanglement and topological superconductivity in the form of artificial Kitaev chains.
Author Correction
In-plane selective area InSb–Al nanowire quantum networks (Communications Physics, (2020), 3, 1, (59), 10.1038/s42005-020-0324-4)
The Data availability statement of this article has been modified to add the accession link to the raw data. The old Data availability statement read “Materials and data that support the findings of this research are available within the paper. All data are available from the corresponding author upon request”. This has been replaced by “Materials and data that support the findings of this research are available within the paper. The raw data have been deposited at https://zenodo.org/record/4589484#.YEoEOy1Y7Sd”. This has been corrected in both the HTML and PDF version of the article.
Topological superconductivity can be engineered in semiconductors with strong spin-orbit interaction coupled to a superconductor. Experimental advances in this field have often been triggered by the development of new hybrid material systems. Among these, two-dimensional electron gases (2DEGs) are of particular interest due to their inherent design flexibility and scalability. Here, we discuss results on a 2D platform based on a ternary 2DEG (InSbAs) coupled to in situ grown aluminum. The spin-orbit coupling in these 2DEGs can be tuned with the As concentration, reaching values up to 400 meV Å, thus exceeding typical values measured in its binary constituents. In addition to a large Landé g-factor of ∼55 (comparable to that of InSb), we show that the clean superconductor-semiconductor interface leads to a hard induced superconducting gap. Using this new platform, we demonstrate the basic operation of phase-controllable Josephson junctions, superconducting islands, and quasi-1D systems, prototypical device geometries used to study Majorana zero modes.
Strong spin–orbit semiconductor nanowires coupled to a superconductor are predicted to host Majorana zero modes. Exchange (braiding) operations of Majorana modes form the logical gates of a topological quantum computer and require a network of nanowires. Here, we utilize an in-plane selective area growth technique for InSb–Al semiconductor–superconductor nanowire networks. Transport channels, free from extended defects, in InSb nanowire networks are realized on insulating, but heavily mismatched InP (111)B substrates by full relaxation of the lattice mismatch at the nanowire/substrate interface and nucleation of a complete network from a single nucleation site by optimizing the surface diffusion length of the adatoms. Essential quantum transport phenomena for topological quantum computing are demonstrated in these structures including phase-coherence lengths exceeding several micrometers with Aharonov–Bohm oscillations up to five harmonics and a hard superconducting gap accompanied by 2e-periodic Coulomb oscillations with an Al-based Cooper pair island integrated in the nanowire network.