S.L.D. ten Haaf
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Few-site implementations of the Kitaev chain offer a minimal platform to study the emergence and stability of Majorana bound states. Here, we realize two- and three-site chains in semiconducting quantum dots coupled via superconductors, and tune them to the sweet spot where zero-energy Majorana modes appear at the chain ends. We demonstrate control of the superconducting phase through both magnetic field and sweet-spot selection, and fully characterize the excitation spectrum under local and global perturbations. All spectral features are identified using the ideal Kitaev chain model. To assess Majorana localization, we couple the system to an additional quantum dot. The absence of energy splitting at the sweet spot is compatible with high-quality Majorana modes, despite the modest chain size.
Majoranas can be lonely
Engineering the Kitaev chain in a two-dimensional electron gas
These compelling prospects have driven significant experimental efforts over the past decades. While the experimental realization of Majoranas has historically been challenging, recent advances have introduced techniques that allow for the reliable creation of these modes. Notably, the team of Leo Kouwenhoven in Delft pioneered an approach that combines quantum dots with superconductivity to construct a so-called Kitaev chain, providing a systematic method to isolate Majorana modes. In such chains, Majoranas are expected to localize at the edges, appearing as zero-energy excitations in tunneling spectroscopy measurements.
This thesis extends the development of these experimental techniques to a new material platform, with the goal of probing the fundamental properties of Majoranas. To do so, we implement a series of experiments demonstrating the construction of a Kitaev chain in an InSbAs two-dimensional electron gas. As first experiment, we couple two quantum dots to either side of a small semiconducting segment in proximity to a superconductor. In this setup, we demonstrate that elastic co-tunnelling and crossed Andreev reflection can be mediated by an Andreev bound state, that their relative amplitudes can be controlled and that spin-orbit interactions enable spin-triplet processes. Leveraging this system, we show that a minimal two-site Kitaev chain can be created, as evidenced by the study of zero-bias conductance features. Building on these results, we investigate extending the system to implement a three-site Kitaev chain. This allows us to show experimentally that the edges of the system, where Majoranas are expected to appear, have distinct properties from the middle of the system, demonstrating a key property of the Kitaev chain. The results in this thesis hope to provide a solid understanding for creating Majoranas in a two-dimensional system, opening up the path toward more complex configurations and the systematic exploration of Majorana physics. ...
These compelling prospects have driven significant experimental efforts over the past decades. While the experimental realization of Majoranas has historically been challenging, recent advances have introduced techniques that allow for the reliable creation of these modes. Notably, the team of Leo Kouwenhoven in Delft pioneered an approach that combines quantum dots with superconductivity to construct a so-called Kitaev chain, providing a systematic method to isolate Majorana modes. In such chains, Majoranas are expected to localize at the edges, appearing as zero-energy excitations in tunneling spectroscopy measurements.
This thesis extends the development of these experimental techniques to a new material platform, with the goal of probing the fundamental properties of Majoranas. To do so, we implement a series of experiments demonstrating the construction of a Kitaev chain in an InSbAs two-dimensional electron gas. As first experiment, we couple two quantum dots to either side of a small semiconducting segment in proximity to a superconductor. In this setup, we demonstrate that elastic co-tunnelling and crossed Andreev reflection can be mediated by an Andreev bound state, that their relative amplitudes can be controlled and that spin-orbit interactions enable spin-triplet processes. Leveraging this system, we show that a minimal two-site Kitaev chain can be created, as evidenced by the study of zero-bias conductance features. Building on these results, we investigate extending the system to implement a three-site Kitaev chain. This allows us to show experimentally that the edges of the system, where Majoranas are expected to appear, have distinct properties from the middle of the system, demonstrating a key property of the Kitaev chain. The results in this thesis hope to provide a solid understanding for creating Majoranas in a two-dimensional system, opening up the path toward more complex configurations and the systematic exploration of Majorana physics.
In semiconducting-superconducting hybrid devices, Andreev bound states (ABSs) can mediate the coupling between quantum dots, allowing for the realization of artificial Kitaev chains. In order to engineer Majorana bound states (MBSs) in these systems, one must control the energy of the ABSs. In this Letter, we show how extended ABSs in a flux-tunable Josephson junction can be used to control the coupling between distant quantum dots separated by ≃1 μm. In particular, we demonstrate that the combination of electrostatic control and phase control over the ABSs increases the parameter space in which MBSs are observed. Finally, by employing an additional spectroscopic probe in the hybrid region between the quantum dots, we gain information about the spatial distribution of the Majorana wave function in a two-site Kitaev chain.
Quantum-dot-superconductor arrays have emerged as a new and promising material platform for realizing topological Kitaev chains. So far, experiments have implemented a two-site chain with limited protection. Here, we propose an experimentally feasible protocol for scaling up the chain in order to enhance the protection of the Majorana zero modes. To this end, we make use of the fact that the relative sign of normal and superconducting hoppings mediated by an Andreev bound state can be changed by electrostatic gates. In this way, our method only relies on the use of individual electrostatic gates on hybrid regions, quantum dots, and tunnel barriers, respectively, without the need for individual magnetic flux control, greatly simplifying the device design. Our work provides guidance for realizing a topologically protected Kitaev chain, which is the building block of error-resilient topological quantum computation.
The formation of a topological superconducting phase in a quantum-dot-based Kitaev chain requires nearest neighbor crossed Andreev reflection and elastic cotunneling. Here, we report on a hybrid InSb nanowire in a three-site Kitaev chain geometry - the smallest system with well-defined bulk and edge - where two superconductor-semiconductor hybrids separate three quantum dots. We demonstrate pairwise crossed Andreev reflection and elastic cotunneling between both pairs of neighboring dots and show sequential tunneling processes involving all three quantum dots. These results are the next step toward the realization of topological superconductivity in long Kitaev chain devices with many coupled quantum dots.
Connecting double quantum dots via a semiconductor-superconductor hybrid segment offers a platform for creating a two-site Kitaev chain that hosts Majorana zero modes at a finely tuned sweet spot. However, the effective couplings mediated by Andreev bound states in the hybrid are generally weak in the tunneling regime. As a consequence, the excitation gap is limited in size, presenting a formidable challenge for using this platform to demonstrate non-Abelian statistics and realize topological quantum computing. Here we systematically study the effects of increasing the dot-hybrid coupling. In particular, the proximity effect transforms the dot orbitals into Yu-Shiba-Rusinov states, and as the coupling strength increases, the excitation gap is significantly enhanced and sensitivity to local perturbation is reduced. We also discuss how the strong-coupling regime shows in experimentally accessible quantities, such as conductance, and provide a protocol for tuning a double-dot system into a sweet spot with a large excitation gap.
Cooper pairs occupy the ground state of superconductors and are typically composed of maximally entangled electrons with opposite spin. In order to study the spin and entanglement properties of these electrons, one must separate them spatially via a process known as Cooper pair splitting (CPS). Here we provide the first demonstration of CPS in a semiconductor two-dimensional electron gas (2DEG). By coupling two quantum dots to a superconductor-semiconductor hybrid region we achieve efficient Cooper pair splitting, and clearly distinguish it from other local and non-local processes. When the spin degeneracy of the dots is lifted, they can be operated as spin-filters to obtain information about the spin of the electrons forming the Cooper pair. Not only do we observe a near perfect splitting of Cooper pairs into opposite-spin electrons (i.e. conventional singlet pairing), but also into equal-spin electrons, thus achieving triplet correlations between the quantum dots. Importantly, the exceptionally large spin-orbit interaction in our 2DEGs results in a strong triplet component, comparable in amplitude to the singlet pairing. The demonstration of CPS in a scalable and flexible platform provides a credible route to study on-chip entanglement and topological superconductivity in the form of artificial Kitaev chains.
A short superconducting segment can couple attached quantum dots via elastic cotunneling (ECT) and crossed Andreev reflection (CAR). Such coupled quantum dots can host Majorana bound states provided that the ratio between CAR and ECT can be controlled. Metallic superconductors have so far been shown to mediate such tunneling phenomena, albeit with limited tunability. Here, we show that Andreev bound states formed in semiconductor-superconductor heterostructures can mediate CAR and ECT over mesoscopic length scales. Andreev bound states possess both an electron and a hole component, giving rise to an intricate interference phenomenon that allows us to tune the ratio between CAR and ECT deterministically. We further show that the combination of intrinsic spin-orbit coupling in InSb nanowires and an applied magnetic field provides another efficient knob to tune the ratio between ECT and CAR and optimize the amount of coupling between neighboring quantum dots.
Majorana bound states constitute one of the simplest examples of emergent non-Abelian excitations in condensed matter physics. A toy model proposed by Kitaev shows that such states can arise at the ends of a spinless p-wave superconducting chain1. Practical proposals for its realization2,3 require coupling neighbouring quantum dots (QDs) in a chain through both electron tunnelling and crossed Andreev reflection4. Although both processes have been observed in semiconducting nanowires and carbon nanotubes5–8, crossed-Andreev interaction was neither easily tunable nor strong enough to induce coherent hybridization of dot states. Here we demonstrate the simultaneous presence of all necessary ingredients for an artificial Kitaev chain: two spin-polarized QDs in an InSb nanowire strongly coupled by both elastic co-tunnelling (ECT) and crossed Andreev reflection (CAR). We fine-tune this system to a sweet spot where a pair of poor man’s Majorana states is predicted to appear. At this sweet spot, the transport characteristics satisfy the theoretical predictions for such a system, including pairwise correlation, zero charge and stability against local perturbations. Although the simple system presented here can be scaled to simulate a full Kitaev chain with an emergent topological order, it can also be used imminently to explore relevant physics related to non-Abelian anyons.
In most naturally occurring superconductors, electrons with opposite spins form Cooper pairs. This includes both conventional s-wave superconductors such as aluminium, as well as high-transition-temperature, d-wave superconductors. Materials with intrinsic p-wave superconductivity, hosting Cooper pairs made of equal-spin electrons, have not been conclusively identified, nor synthesized, despite promising progress1–3. Instead, engineered platforms where s-wave superconductors are brought into contact with magnetic materials have shown convincing signatures of equal-spin pairing4–6. Here we directly measure equal-spin pairing between spin-polarized quantum dots. This pairing is proximity-induced from an s-wave superconductor into a semiconducting nanowire with strong spin–orbit interaction. We demonstrate such pairing by showing that breaking a Cooper pair can result in two electrons with equal spin polarization. Our results demonstrate controllable detection of singlet and triplet pairing between the quantum dots. Achieving such triplet pairing in a sequence of quantum dots will be required for realizing an artificial Kitaev chain7–9.